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Radiation resistance of single and multilayer coatings against synchrotron radiation

Research output: Chapter in book/report/conference proceedingConference contributionResearchpeer review

Authors

  • Stefan Günster
  • Holger Blaschke
  • Detlev Ristau
  • Miltcho Boyanov Danailov

External Research Organisations

  • Laser Zentrum Hannover e.V. (LZH)
  • Sincrotrone Trieste
  • Fraunhofer Institute for Applied Optics and Precision Engineering (IOF)
  • Ente Per Le Nuove Tecnologie L'energia e l'ambiente

Details

Original languageEnglish
Title of host publicationAdvances in Optical Thin Films
Subtitle of host publication30 September - 3 October 2003, St. Etienne, France
Place of PublicationBellingham
PublisherSPIE
Pages146-157
Number of pages12
ISBN (print)0-8194-5134-7
Publication statusPublished - 25 Feb 2004
Externally publishedYes
EventAdvances in Optical Thin Films - St. Etienne, France
Duration: 30 Sept 20033 Oct 2003

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
PublisherSPIE
Volume5250
ISSN (Print)0277-786X

Abstract

Optical coatings for the use in free electron laser systems have to withstand high power laser radiation and the intense energetic background radiation of the synchrotron radiation source. In general, the bombardment with high energetic photons leads to irreversible changes and a discoloration of the specimen. For the development of appropriate optical coatings, the degradation mechanisms of available optical materials have to be characterized. In this contribution the degradation mechanisms of single layer coatings (fluoride and oxide materials) and multilayer systems will be presented. Fluoride and oxide single layers were produced by thermal evaporation and high energetic ion beam sputter deposition. The same methods were employed for the deposition of multilayer systems. High reflecting coatings for the wavelength region around 180nm were chosen for the irradiation tests. All samples were characterized after production by spectrophotometry covering the VUV, VIS, and MIR spectral range. Mechanical coating stress was evaluated with interferometric methods. Synchrotron irradiation tests were performed at ELETTRA, using a standardized irradiation cycle for all tests. Ambient pressure and possible contamination in the vacuum environment were monitored by mass spectrometry. For comparison, the optical coatings were investigated again in the VUV, VIS, and MIR spectral range after irradiation. On selected samples XRD measurements were performed. The observed degradation mechanisms comprise severe damages like coating and substrate surface ablation. Color centre formation in the VIS spectral range and an increase of VUV absorption were found as a major origin for a severe degradation of VUV transmittance On the basis of the performed investigations, a selection of coating materials and coating systems is possible in respect to the damage effects caused by synchrotron radiation.

Keywords

    Optics characterization, Radiation resistance, Synchrotron radiation, VUV coatings

ASJC Scopus subject areas

Cite this

Radiation resistance of single and multilayer coatings against synchrotron radiation. / Günster, Stefan; Blaschke, Holger; Ristau, Detlev et al.
Advances in Optical Thin Films: 30 September - 3 October 2003, St. Etienne, France. Bellingham: SPIE, 2004. p. 146-157 (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 5250).

Research output: Chapter in book/report/conference proceedingConference contributionResearchpeer review

Günster, S, Blaschke, H, Ristau, D, Danailov, MB, Trovó, M, Gatto, A, Kaiser, N, Sarto, F, Flori, D & Menchini, F 2004, Radiation resistance of single and multilayer coatings against synchrotron radiation. in Advances in Optical Thin Films: 30 September - 3 October 2003, St. Etienne, France. Proceedings of SPIE - The International Society for Optical Engineering, vol. 5250, SPIE, Bellingham, pp. 146-157, Advances in Optical Thin Films, St. Etienne, France, 30 Sept 2003. https://doi.org/10.1117/12.514801
Günster, S., Blaschke, H., Ristau, D., Danailov, M. B., Trovó, M., Gatto, A., Kaiser, N., Sarto, F., Flori, D., & Menchini, F. (2004). Radiation resistance of single and multilayer coatings against synchrotron radiation. In Advances in Optical Thin Films: 30 September - 3 October 2003, St. Etienne, France (pp. 146-157). (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 5250). SPIE. https://doi.org/10.1117/12.514801
Günster S, Blaschke H, Ristau D, Danailov MB, Trovó M, Gatto A et al. Radiation resistance of single and multilayer coatings against synchrotron radiation. In Advances in Optical Thin Films: 30 September - 3 October 2003, St. Etienne, France. Bellingham: SPIE. 2004. p. 146-157. (Proceedings of SPIE - The International Society for Optical Engineering). doi: 10.1117/12.514801
Günster, Stefan ; Blaschke, Holger ; Ristau, Detlev et al. / Radiation resistance of single and multilayer coatings against synchrotron radiation. Advances in Optical Thin Films: 30 September - 3 October 2003, St. Etienne, France. Bellingham : SPIE, 2004. pp. 146-157 (Proceedings of SPIE - The International Society for Optical Engineering).
Download
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T1 - Radiation resistance of single and multilayer coatings against synchrotron radiation

AU - Günster, Stefan

AU - Blaschke, Holger

AU - Ristau, Detlev

AU - Danailov, Miltcho Boyanov

AU - Trovó, Mauro

AU - Gatto, Alexandre

AU - Kaiser, Norbert

AU - Sarto, Fransesca

AU - Flori, Daniel

AU - Menchini, F.

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N2 - Optical coatings for the use in free electron laser systems have to withstand high power laser radiation and the intense energetic background radiation of the synchrotron radiation source. In general, the bombardment with high energetic photons leads to irreversible changes and a discoloration of the specimen. For the development of appropriate optical coatings, the degradation mechanisms of available optical materials have to be characterized. In this contribution the degradation mechanisms of single layer coatings (fluoride and oxide materials) and multilayer systems will be presented. Fluoride and oxide single layers were produced by thermal evaporation and high energetic ion beam sputter deposition. The same methods were employed for the deposition of multilayer systems. High reflecting coatings for the wavelength region around 180nm were chosen for the irradiation tests. All samples were characterized after production by spectrophotometry covering the VUV, VIS, and MIR spectral range. Mechanical coating stress was evaluated with interferometric methods. Synchrotron irradiation tests were performed at ELETTRA, using a standardized irradiation cycle for all tests. Ambient pressure and possible contamination in the vacuum environment were monitored by mass spectrometry. For comparison, the optical coatings were investigated again in the VUV, VIS, and MIR spectral range after irradiation. On selected samples XRD measurements were performed. The observed degradation mechanisms comprise severe damages like coating and substrate surface ablation. Color centre formation in the VIS spectral range and an increase of VUV absorption were found as a major origin for a severe degradation of VUV transmittance On the basis of the performed investigations, a selection of coating materials and coating systems is possible in respect to the damage effects caused by synchrotron radiation.

AB - Optical coatings for the use in free electron laser systems have to withstand high power laser radiation and the intense energetic background radiation of the synchrotron radiation source. In general, the bombardment with high energetic photons leads to irreversible changes and a discoloration of the specimen. For the development of appropriate optical coatings, the degradation mechanisms of available optical materials have to be characterized. In this contribution the degradation mechanisms of single layer coatings (fluoride and oxide materials) and multilayer systems will be presented. Fluoride and oxide single layers were produced by thermal evaporation and high energetic ion beam sputter deposition. The same methods were employed for the deposition of multilayer systems. High reflecting coatings for the wavelength region around 180nm were chosen for the irradiation tests. All samples were characterized after production by spectrophotometry covering the VUV, VIS, and MIR spectral range. Mechanical coating stress was evaluated with interferometric methods. Synchrotron irradiation tests were performed at ELETTRA, using a standardized irradiation cycle for all tests. Ambient pressure and possible contamination in the vacuum environment were monitored by mass spectrometry. For comparison, the optical coatings were investigated again in the VUV, VIS, and MIR spectral range after irradiation. On selected samples XRD measurements were performed. The observed degradation mechanisms comprise severe damages like coating and substrate surface ablation. Color centre formation in the VIS spectral range and an increase of VUV absorption were found as a major origin for a severe degradation of VUV transmittance On the basis of the performed investigations, a selection of coating materials and coating systems is possible in respect to the damage effects caused by synchrotron radiation.

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