Engineering Nanoparticles with Pure High-Order Multipole Scattering

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Vladimir A. Zenin
  • Cesar E. Garcia-Ortiz
  • Andrey B. Evlyukhin
  • Yuanqing Yang
  • Radu Malureanu
  • Sergey M. Novikov
  • Victor Coello
  • Boris N. Chichkov
  • Sergey I. Bozhevolnyi
  • Andrei V. Lavrinenko
  • N. Asger Mortensen

External Research Organisations

  • Centro de Investigacion Cientifica y de Educacion Superior de Ensenada
  • Moscow Institute of Physics and Technology
  • Technical University of Denmark
  • Lebedev Physical Institute of the Russian Academy of Sciences (LPI RAS)
  • University of Southern Denmark
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Details

Original languageEnglish
Pages (from-to)1067-1075
Number of pages9
JournalACS PHOTONICS
Volume7
Issue number4
Publication statusPublished - 28 Feb 2020

Abstract

The ability to control scattering directionality of nanoparticles is in high demand for many nanophotonic applications. One of the challenges is to design nanoparticles producing pure high-order multipole scattering (e.g., octopole, hexadecapole), whose contribution is usually negligible compared with strong low-order multipole scattering (i.e., dipole or quadrupole). Here we present an intuitive way to design such nanoparticles by introducing a void inside them. We show that both shell and ring nanostructures allow regimes with nearly pure high-order multipole scattering. Experimentally measured scattering diagrams from properly designed silicon rings at near-infrared wavelengths (∼800 nm) reproduce well scattering patterns of an electric octopole and magnetic hexadecapole. Our findings advance significantly inverse engineering of nanoparticles from given complex scattering characteristics, with possible applications in biosensing, optical metasurfaces, and quantum communications.

Keywords

    all-dielectric nanoparticles, hexadecapole, multipole decomposition, octopole, scattering diagram

ASJC Scopus subject areas

Cite this

Engineering Nanoparticles with Pure High-Order Multipole Scattering. / Zenin, Vladimir A.; Garcia-Ortiz, Cesar E.; Evlyukhin, Andrey B. et al.
In: ACS PHOTONICS, Vol. 7, No. 4, 28.02.2020, p. 1067-1075.

Research output: Contribution to journalArticleResearchpeer review

Zenin, VA, Garcia-Ortiz, CE, Evlyukhin, AB, Yang, Y, Malureanu, R, Novikov, SM, Coello, V, Chichkov, BN, Bozhevolnyi, SI, Lavrinenko, AV & Mortensen, NA 2020, 'Engineering Nanoparticles with Pure High-Order Multipole Scattering', ACS PHOTONICS, vol. 7, no. 4, pp. 1067-1075. https://doi.org/10.1021/acsphotonics.0c00078
Zenin, V. A., Garcia-Ortiz, C. E., Evlyukhin, A. B., Yang, Y., Malureanu, R., Novikov, S. M., Coello, V., Chichkov, B. N., Bozhevolnyi, S. I., Lavrinenko, A. V., & Mortensen, N. A. (2020). Engineering Nanoparticles with Pure High-Order Multipole Scattering. ACS PHOTONICS, 7(4), 1067-1075. https://doi.org/10.1021/acsphotonics.0c00078
Zenin VA, Garcia-Ortiz CE, Evlyukhin AB, Yang Y, Malureanu R, Novikov SM et al. Engineering Nanoparticles with Pure High-Order Multipole Scattering. ACS PHOTONICS. 2020 Feb 28;7(4):1067-1075. doi: 10.1021/acsphotonics.0c00078
Zenin, Vladimir A. ; Garcia-Ortiz, Cesar E. ; Evlyukhin, Andrey B. et al. / Engineering Nanoparticles with Pure High-Order Multipole Scattering. In: ACS PHOTONICS. 2020 ; Vol. 7, No. 4. pp. 1067-1075.
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@article{bad6c09bef654f0d96723c90292be233,
title = "Engineering Nanoparticles with Pure High-Order Multipole Scattering",
abstract = "The ability to control scattering directionality of nanoparticles is in high demand for many nanophotonic applications. One of the challenges is to design nanoparticles producing pure high-order multipole scattering (e.g., octopole, hexadecapole), whose contribution is usually negligible compared with strong low-order multipole scattering (i.e., dipole or quadrupole). Here we present an intuitive way to design such nanoparticles by introducing a void inside them. We show that both shell and ring nanostructures allow regimes with nearly pure high-order multipole scattering. Experimentally measured scattering diagrams from properly designed silicon rings at near-infrared wavelengths (∼800 nm) reproduce well scattering patterns of an electric octopole and magnetic hexadecapole. Our findings advance significantly inverse engineering of nanoparticles from given complex scattering characteristics, with possible applications in biosensing, optical metasurfaces, and quantum communications.",
keywords = "all-dielectric nanoparticles, hexadecapole, multipole decomposition, octopole, scattering diagram",
author = "Zenin, {Vladimir A.} and Garcia-Ortiz, {Cesar E.} and Evlyukhin, {Andrey B.} and Yuanqing Yang and Radu Malureanu and Novikov, {Sergey M.} and Victor Coello and Chichkov, {Boris N.} and Bozhevolnyi, {Sergey I.} and Lavrinenko, {Andrei V.} and Mortensen, {N. Asger}",
note = "The authors acknowledge financial support from the European Research Council (the PLAQNAP project, Grant No. 341054) and the University of Southern Denmark (SDU2020 funding), from scholarship 299967. N.A.M. is a VILLUM Investigator supported by Villum Fonden (Grant No. 16498). C.E.G.-O and V.C. acknowledge the technical assistance of Fabiola Armenta with the experimental setup. V.C. and C.E.G.-O. acknowledge funding from CONACYT Basic Scientific Research Grants No. 250719 and No. 252621. RM and AVL acknowledge the financial support from Villum Fonden ”DarkSILD project” (Grant No. 11116) as well as the support of the National Centre for Nano Fabrication and Characterization (DTU Nanolab) for fabrication of the structures. A.B.E. and B.N.C. acknowledge financial support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany{\textquoteright}s Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122, Project No. 390833453), the Cluster of Excellence QuantumFrontiers (EXC 2123, Project No. 390837967), and DFG Project CH179/34-1. Numerical simulation was partially supported by the Russian Science Foundation (Grant No. 18-19-00684).",
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T1 - Engineering Nanoparticles with Pure High-Order Multipole Scattering

AU - Zenin, Vladimir A.

AU - Garcia-Ortiz, Cesar E.

AU - Evlyukhin, Andrey B.

AU - Yang, Yuanqing

AU - Malureanu, Radu

AU - Novikov, Sergey M.

AU - Coello, Victor

AU - Chichkov, Boris N.

AU - Bozhevolnyi, Sergey I.

AU - Lavrinenko, Andrei V.

AU - Mortensen, N. Asger

N1 - The authors acknowledge financial support from the European Research Council (the PLAQNAP project, Grant No. 341054) and the University of Southern Denmark (SDU2020 funding), from scholarship 299967. N.A.M. is a VILLUM Investigator supported by Villum Fonden (Grant No. 16498). C.E.G.-O and V.C. acknowledge the technical assistance of Fabiola Armenta with the experimental setup. V.C. and C.E.G.-O. acknowledge funding from CONACYT Basic Scientific Research Grants No. 250719 and No. 252621. RM and AVL acknowledge the financial support from Villum Fonden ”DarkSILD project” (Grant No. 11116) as well as the support of the National Centre for Nano Fabrication and Characterization (DTU Nanolab) for fabrication of the structures. A.B.E. and B.N.C. acknowledge financial support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany’s Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122, Project No. 390833453), the Cluster of Excellence QuantumFrontiers (EXC 2123, Project No. 390837967), and DFG Project CH179/34-1. Numerical simulation was partially supported by the Russian Science Foundation (Grant No. 18-19-00684).

PY - 2020/2/28

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N2 - The ability to control scattering directionality of nanoparticles is in high demand for many nanophotonic applications. One of the challenges is to design nanoparticles producing pure high-order multipole scattering (e.g., octopole, hexadecapole), whose contribution is usually negligible compared with strong low-order multipole scattering (i.e., dipole or quadrupole). Here we present an intuitive way to design such nanoparticles by introducing a void inside them. We show that both shell and ring nanostructures allow regimes with nearly pure high-order multipole scattering. Experimentally measured scattering diagrams from properly designed silicon rings at near-infrared wavelengths (∼800 nm) reproduce well scattering patterns of an electric octopole and magnetic hexadecapole. Our findings advance significantly inverse engineering of nanoparticles from given complex scattering characteristics, with possible applications in biosensing, optical metasurfaces, and quantum communications.

AB - The ability to control scattering directionality of nanoparticles is in high demand for many nanophotonic applications. One of the challenges is to design nanoparticles producing pure high-order multipole scattering (e.g., octopole, hexadecapole), whose contribution is usually negligible compared with strong low-order multipole scattering (i.e., dipole or quadrupole). Here we present an intuitive way to design such nanoparticles by introducing a void inside them. We show that both shell and ring nanostructures allow regimes with nearly pure high-order multipole scattering. Experimentally measured scattering diagrams from properly designed silicon rings at near-infrared wavelengths (∼800 nm) reproduce well scattering patterns of an electric octopole and magnetic hexadecapole. Our findings advance significantly inverse engineering of nanoparticles from given complex scattering characteristics, with possible applications in biosensing, optical metasurfaces, and quantum communications.

KW - all-dielectric nanoparticles

KW - hexadecapole

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JO - ACS PHOTONICS

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