Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Autoren

  • Franziska Lübkemann
  • Jan Frederick Miethe
  • Frank Steinbach
  • Pascal Rusch
  • Anja Schlosser
  • Dániel Zámbó
  • Thea Heinemeyer
  • Dominik Natke
  • Dorian Zok
  • Dirk Dorfs
  • Nadja C. Bigall
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Details

OriginalspracheEnglisch
Aufsatznummer1902186
FachzeitschriftSMALL
Jahrgang15
Ausgabenummer39
PublikationsstatusVeröffentlicht - 25 Sept. 2019

Abstract

Nanoparticle-based voluminous 3D networks with low densities are a unique class of materials and are commonly known as aerogels. Due to the high surface-to-volume ratio, aerogels and xerogels might be suitable materials for applications in different fields, e.g. photocatalysis, catalysis, or sensing. One major difficulty in the handling of nanoparticle-based aerogels and xerogels is the defined patterning of these structures on different substrates and surfaces. The automated manufacturing of nanoparticle-based aerogel- or xerogel-coated electrodes can easily be realized via inkjet printing. The main focus of this work is the implementation of the standard nanoparticle-based gelation process in a commercial inkjet printing system. By simultaneously printing semiconductor nanoparticles and a destabilization agent, a 3D network on a conducting and transparent surface is obtained. First spectro-electrochemical measurements are recorded to investigate the charge–carrier mobility within these 3D semiconductor-based xerogel networks.

ASJC Scopus Sachgebiete

Zitieren

Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing. / Lübkemann, Franziska; Miethe, Jan Frederick; Steinbach, Frank et al.
in: SMALL, Jahrgang 15, Nr. 39, 1902186, 25.09.2019.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

Lübkemann, F, Miethe, JF, Steinbach, F, Rusch, P, Schlosser, A, Zámbó, D, Heinemeyer, T, Natke, D, Zok, D, Dorfs, D & Bigall, NC 2019, 'Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing', SMALL, Jg. 15, Nr. 39, 1902186. https://doi.org/10.1002/smll.201902186
Lübkemann, F., Miethe, J. F., Steinbach, F., Rusch, P., Schlosser, A., Zámbó, D., Heinemeyer, T., Natke, D., Zok, D., Dorfs, D., & Bigall, N. C. (2019). Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing. SMALL, 15(39), Artikel 1902186. https://doi.org/10.1002/smll.201902186
Lübkemann F, Miethe JF, Steinbach F, Rusch P, Schlosser A, Zámbó D et al. Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing. SMALL. 2019 Sep 25;15(39):1902186. doi: 10.1002/smll.201902186
Lübkemann, Franziska ; Miethe, Jan Frederick ; Steinbach, Frank et al. / Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing. in: SMALL. 2019 ; Jahrgang 15, Nr. 39.
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abstract = "Nanoparticle-based voluminous 3D networks with low densities are a unique class of materials and are commonly known as aerogels. Due to the high surface-to-volume ratio, aerogels and xerogels might be suitable materials for applications in different fields, e.g. photocatalysis, catalysis, or sensing. One major difficulty in the handling of nanoparticle-based aerogels and xerogels is the defined patterning of these structures on different substrates and surfaces. The automated manufacturing of nanoparticle-based aerogel- or xerogel-coated electrodes can easily be realized via inkjet printing. The main focus of this work is the implementation of the standard nanoparticle-based gelation process in a commercial inkjet printing system. By simultaneously printing semiconductor nanoparticles and a destabilization agent, a 3D network on a conducting and transparent surface is obtained. First spectro-electrochemical measurements are recorded to investigate the charge–carrier mobility within these 3D semiconductor-based xerogel networks.",
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note = "Funding information: The authors (N.C.B., F.L., J.F.M.) are grateful for financial support from the German Federal Ministry of Education and Research (BMBF) within the framework of the program NanoMatFutur, support code 03X5525. Furthermore, the project leading to these results has in part received funding from the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation program (grant agreement No. 714429). The authors (D.D. and F.L.) are grateful for the financial support from Volkswagen foundation (lower Saxony/Israel cooperation, Grant ZN2916). The author D.D. thanks the DFG (research Grant 1580/5-1). The author N.C.B. thanks the DFG (research Grant BI 1708/4-1). The project has in parts been funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122). The author A.S. thanks the Hannover school of nanotechnology for financial support. The authors thank Prof. Caro and Prof. Feldhoff for access to a scanning electron microscope and the Laboratory of Nano and Quantum Engineering for support.",
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T1 - Patterning of Nanoparticle-Based Aerogels and Xerogels by Inkjet Printing

AU - Lübkemann, Franziska

AU - Miethe, Jan Frederick

AU - Steinbach, Frank

AU - Rusch, Pascal

AU - Schlosser, Anja

AU - Zámbó, Dániel

AU - Heinemeyer, Thea

AU - Natke, Dominik

AU - Zok, Dorian

AU - Dorfs, Dirk

AU - Bigall, Nadja C.

N1 - Funding information: The authors (N.C.B., F.L., J.F.M.) are grateful for financial support from the German Federal Ministry of Education and Research (BMBF) within the framework of the program NanoMatFutur, support code 03X5525. Furthermore, the project leading to these results has in part received funding from the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation program (grant agreement No. 714429). The authors (D.D. and F.L.) are grateful for the financial support from Volkswagen foundation (lower Saxony/Israel cooperation, Grant ZN2916). The author D.D. thanks the DFG (research Grant 1580/5-1). The author N.C.B. thanks the DFG (research Grant BI 1708/4-1). The project has in parts been funded by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122). The author A.S. thanks the Hannover school of nanotechnology for financial support. The authors thank Prof. Caro and Prof. Feldhoff for access to a scanning electron microscope and the Laboratory of Nano and Quantum Engineering for support.

PY - 2019/9/25

Y1 - 2019/9/25

N2 - Nanoparticle-based voluminous 3D networks with low densities are a unique class of materials and are commonly known as aerogels. Due to the high surface-to-volume ratio, aerogels and xerogels might be suitable materials for applications in different fields, e.g. photocatalysis, catalysis, or sensing. One major difficulty in the handling of nanoparticle-based aerogels and xerogels is the defined patterning of these structures on different substrates and surfaces. The automated manufacturing of nanoparticle-based aerogel- or xerogel-coated electrodes can easily be realized via inkjet printing. The main focus of this work is the implementation of the standard nanoparticle-based gelation process in a commercial inkjet printing system. By simultaneously printing semiconductor nanoparticles and a destabilization agent, a 3D network on a conducting and transparent surface is obtained. First spectro-electrochemical measurements are recorded to investigate the charge–carrier mobility within these 3D semiconductor-based xerogel networks.

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