Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators

Research output: Contribution to journalArticleResearchpeer review

Authors

  • Rana Nicolas
  • Liping Shi
  • Bruno Chanteau
  • Dominik Franz
  • Maria Kholodstova
  • Quentin Ripault
  • José R.C. Andrade
  • Bianca Iwan
  • Willem Boutu
  • Milutin Kovacev
  • Hamed Merdji
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Details

Original languageEnglish
Pages (from-to)1883-1889
Number of pages7
JournalPlasmonics
Volume16
Issue number6
Early online date29 Apr 2021
Publication statusPublished - Dec 2021

Abstract

Enhancing ultrafast nonlinear processes at a nanometer scale has the potential of creating novel nano-sources of energetic photons or particles useful for many applications, especially for embedded diagnostics. In this work, we investigate the plasmonic amplification of the third harmonic generation (THG) from a metal-dielectric-metal (MDM) nano-resonator in the near-terawatt intensity regime. In our geometry, the Fabry-Pérot plasmonic resonator reaches a high local enhancement of the laser electric field over a large volume of a SiO2 dielectric film. The THG signal is amplified by more than one order of magnitude, with a higher efficiency compared to previous plasmonic geometries. The polarization dependence with respect to the fundamental laser allows an ON/OFF switch of the THG enhancement in the nanostructures which is a strong signature of the plasmonic origin of the THG amplification. Furthermore, the dispersion scan shows that the third harmonic spectrum is strongly redshifted with respect to the peak of its linear extinction spectrum. Using the nonlinear anharmonic model, we confirm that the third harmonic behavior dominantly arises from the silica layer.

Keywords

    Metal-dielectric-metal metasurface, Nonlinear anharmonic model, Plasmonic resonance, Third harmonic generation

ASJC Scopus subject areas

  • Biochemistry, Genetics and Molecular Biology(all)
  • Biotechnology
  • Biochemistry, Genetics and Molecular Biology(all)
  • Biophysics
  • Biochemistry, Genetics and Molecular Biology(all)
  • Biochemistry

Cite this

Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators. / Nicolas, Rana; Shi, Liping; Chanteau, Bruno et al.
In: Plasmonics, Vol. 16, No. 6, 12.2021, p. 1883-1889.

Research output: Contribution to journalArticleResearchpeer review

Nicolas, R, Shi, L, Chanteau, B, Franz, D, Kholodstova, M, Ripault, Q, Andrade, JRC, Iwan, B, Boutu, W, Kovacev, M & Merdji, H 2021, 'Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators', Plasmonics, vol. 16, no. 6, pp. 1883-1889. https://doi.org/10.1007/s11468-021-01444-3
Nicolas, R., Shi, L., Chanteau, B., Franz, D., Kholodstova, M., Ripault, Q., Andrade, J. R. C., Iwan, B., Boutu, W., Kovacev, M., & Merdji, H. (2021). Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators. Plasmonics, 16(6), 1883-1889. https://doi.org/10.1007/s11468-021-01444-3
Nicolas R, Shi L, Chanteau B, Franz D, Kholodstova M, Ripault Q et al. Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators. Plasmonics. 2021 Dec;16(6):1883-1889. Epub 2021 Apr 29. doi: 10.1007/s11468-021-01444-3
Nicolas, Rana ; Shi, Liping ; Chanteau, Bruno et al. / Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators. In: Plasmonics. 2021 ; Vol. 16, No. 6. pp. 1883-1889.
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title = "Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators",
abstract = "Enhancing ultrafast nonlinear processes at a nanometer scale has the potential of creating novel nano-sources of energetic photons or particles useful for many applications, especially for embedded diagnostics. In this work, we investigate the plasmonic amplification of the third harmonic generation (THG) from a metal-dielectric-metal (MDM) nano-resonator in the near-terawatt intensity regime. In our geometry, the Fabry-P{\'e}rot plasmonic resonator reaches a high local enhancement of the laser electric field over a large volume of a SiO2 dielectric film. The THG signal is amplified by more than one order of magnitude, with a higher efficiency compared to previous plasmonic geometries. The polarization dependence with respect to the fundamental laser allows an ON/OFF switch of the THG enhancement in the nanostructures which is a strong signature of the plasmonic origin of the THG amplification. Furthermore, the dispersion scan shows that the third harmonic spectrum is strongly redshifted with respect to the peak of its linear extinction spectrum. Using the nonlinear anharmonic model, we confirm that the third harmonic behavior dominantly arises from the silica layer.",
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author = "Rana Nicolas and Liping Shi and Bruno Chanteau and Dominik Franz and Maria Kholodstova and Quentin Ripault and Andrade, {Jos{\'e} R.C.} and Bianca Iwan and Willem Boutu and Milutin Kovacev and Hamed Merdji",
note = "Funding Information: We received financial support from the European Union through the Future and Emerging Technologies (FET) Open H2020: PETACom (grant 829153), OPTOLOGIC (grant 899794). Support from the DGA RAPID grant “SWIM,” from the Centre National de Comp{\'e}tences en Nanosciences (C{\textquoteright}NANO) research program through the NanoscopiX grant; the LABoratoire d{\textquoteright}EXcelence Physique Atoms Lumi{\`e}re Mati{\`e}re—LABEX PALM (ANR-10-LABX-0039-PALM), through the grants “Plasmon-X” and “STAMPS” and, finally, the Action de Soutien {\`a} la Technologie et {\`a} la Recherche en Essonne (ASTRE) program through the “NanoLight” grant are also acknowledged. Support from the French National Research Agency through the PACHA grant (ANR-17-CE30-0008–01). Financial support by the German Research Foundation, grant KO 3798/4–1 and from Germany{\textquoteright}s Excellence Strategy EXC-2123 and Germany{\textquoteright}s Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122, Project ID 390833453), Lower Saxony through “Quanten und Nanometrologie” (QUANOMET, Project Nanophotonik). ",
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T1 - Plasmon-Amplified Third Harmonic Generation in Metal/Dielectric Resonators

AU - Nicolas, Rana

AU - Shi, Liping

AU - Chanteau, Bruno

AU - Franz, Dominik

AU - Kholodstova, Maria

AU - Ripault, Quentin

AU - Andrade, José R.C.

AU - Iwan, Bianca

AU - Boutu, Willem

AU - Kovacev, Milutin

AU - Merdji, Hamed

N1 - Funding Information: We received financial support from the European Union through the Future and Emerging Technologies (FET) Open H2020: PETACom (grant 829153), OPTOLOGIC (grant 899794). Support from the DGA RAPID grant “SWIM,” from the Centre National de Compétences en Nanosciences (C’NANO) research program through the NanoscopiX grant; the LABoratoire d’EXcelence Physique Atoms Lumière Matière—LABEX PALM (ANR-10-LABX-0039-PALM), through the grants “Plasmon-X” and “STAMPS” and, finally, the Action de Soutien à la Technologie et à la Recherche en Essonne (ASTRE) program through the “NanoLight” grant are also acknowledged. Support from the French National Research Agency through the PACHA grant (ANR-17-CE30-0008–01). Financial support by the German Research Foundation, grant KO 3798/4–1 and from Germany’s Excellence Strategy EXC-2123 and Germany’s Excellence Strategy within the Cluster of Excellence PhoenixD (EXC 2122, Project ID 390833453), Lower Saxony through “Quanten und Nanometrologie” (QUANOMET, Project Nanophotonik).

PY - 2021/12

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N2 - Enhancing ultrafast nonlinear processes at a nanometer scale has the potential of creating novel nano-sources of energetic photons or particles useful for many applications, especially for embedded diagnostics. In this work, we investigate the plasmonic amplification of the third harmonic generation (THG) from a metal-dielectric-metal (MDM) nano-resonator in the near-terawatt intensity regime. In our geometry, the Fabry-Pérot plasmonic resonator reaches a high local enhancement of the laser electric field over a large volume of a SiO2 dielectric film. The THG signal is amplified by more than one order of magnitude, with a higher efficiency compared to previous plasmonic geometries. The polarization dependence with respect to the fundamental laser allows an ON/OFF switch of the THG enhancement in the nanostructures which is a strong signature of the plasmonic origin of the THG amplification. Furthermore, the dispersion scan shows that the third harmonic spectrum is strongly redshifted with respect to the peak of its linear extinction spectrum. Using the nonlinear anharmonic model, we confirm that the third harmonic behavior dominantly arises from the silica layer.

AB - Enhancing ultrafast nonlinear processes at a nanometer scale has the potential of creating novel nano-sources of energetic photons or particles useful for many applications, especially for embedded diagnostics. In this work, we investigate the plasmonic amplification of the third harmonic generation (THG) from a metal-dielectric-metal (MDM) nano-resonator in the near-terawatt intensity regime. In our geometry, the Fabry-Pérot plasmonic resonator reaches a high local enhancement of the laser electric field over a large volume of a SiO2 dielectric film. The THG signal is amplified by more than one order of magnitude, with a higher efficiency compared to previous plasmonic geometries. The polarization dependence with respect to the fundamental laser allows an ON/OFF switch of the THG enhancement in the nanostructures which is a strong signature of the plasmonic origin of the THG amplification. Furthermore, the dispersion scan shows that the third harmonic spectrum is strongly redshifted with respect to the peak of its linear extinction spectrum. Using the nonlinear anharmonic model, we confirm that the third harmonic behavior dominantly arises from the silica layer.

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