Effect of heat treatment on nanoparticle reinforced Nb-18.7Si alloy

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OriginalspracheEnglisch
Aufsatznummer107170
FachzeitschriftInternational Journal of Refractory Metals and Hard Materials
Jahrgang130
Frühes Online-Datum29 März 2025
PublikationsstatusVeröffentlicht - Aug. 2025

Abstract

Eutectic Nb-18.7Si alloys with different ceramic nanoparticle addition (Al2O3, TiC, SiC, 5 mol.-%), prepared by arc-melting, were heat-treated for 24 h at 1500 °C. Phase composition, microstructure transition and mechanical properties were investigated. The results show that the γ-Nb5Si3 and small Nb3Si phases from the as-cast alloy decomposed into α-Nb5Si3 and Nbss/α-Nb5Si3-eutectoids. Larger Nb3Si phases still existed after heat treatment. Additionally, after heat treatment the Nbss phases were interconnected to a continuous matrix, while silicides appeared coarsened and spherical while being uniformly distributed in the Nbss phase. This effect was most pronounced in the alloy with addition of Al2O3 nanoparticles, due to the ultrafine nano-scale lamellar structures of Nbss + α-Nb5Si3 in its as-cast condition. While the added nanoparticles had a strong effect on the initial microstructure of the as-cast state, they showed no noticeable effects like pinning of grain boundaries during heat treatment. A decrease in hardness was observed due to the coarsening of the microstructure and the reduced area fraction of silicide phases. However, the transformation to the coarser microstructure with a continuous Nbss matrix and spherical silicide phases seems to be effective in inhibiting crack propagation by promoting crack deflection and bridging over the Nbss phase.

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Effect of heat treatment on nanoparticle reinforced Nb-18.7Si alloy. / Holzmann, Elisa; Barienti, Khemais; Guglielmi, Mattia et al.
in: International Journal of Refractory Metals and Hard Materials, Jahrgang 130, 107170, 08.2025.

Publikation: Beitrag in FachzeitschriftArtikelForschungPeer-Review

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title = "Effect of heat treatment on nanoparticle reinforced Nb-18.7Si alloy",
abstract = "Eutectic Nb-18.7Si alloys with different ceramic nanoparticle addition (Al2O3, TiC, SiC, 5 mol.-%), prepared by arc-melting, were heat-treated for 24 h at 1500 °C. Phase composition, microstructure transition and mechanical properties were investigated. The results show that the γ-Nb5Si3 and small Nb3Si phases from the as-cast alloy decomposed into α-Nb5Si3 and Nbss/α-Nb5Si3-eutectoids. Larger Nb3Si phases still existed after heat treatment. Additionally, after heat treatment the Nbss phases were interconnected to a continuous matrix, while silicides appeared coarsened and spherical while being uniformly distributed in the Nbss phase. This effect was most pronounced in the alloy with addition of Al2O3 nanoparticles, due to the ultrafine nano-scale lamellar structures of Nbss + α-Nb5Si3 in its as-cast condition. While the added nanoparticles had a strong effect on the initial microstructure of the as-cast state, they showed no noticeable effects like pinning of grain boundaries during heat treatment. A decrease in hardness was observed due to the coarsening of the microstructure and the reduced area fraction of silicide phases. However, the transformation to the coarser microstructure with a continuous Nbss matrix and spherical silicide phases seems to be effective in inhibiting crack propagation by promoting crack deflection and bridging over the Nbss phase.",
keywords = "AlO, Heat treatment, Microstructure, Nanoparticle, Nb-Si based alloy, SiC, TiC",
author = "Elisa Holzmann and Khemais Barienti and Mattia Guglielmi and Egbert Baake and Sebastian Herbst and Maier, {Hans J{\"u}rgen}",
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journal = "International Journal of Refractory Metals and Hard Materials",
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T1 - Effect of heat treatment on nanoparticle reinforced Nb-18.7Si alloy

AU - Holzmann, Elisa

AU - Barienti, Khemais

AU - Guglielmi, Mattia

AU - Baake, Egbert

AU - Herbst, Sebastian

AU - Maier, Hans Jürgen

N1 - Publisher Copyright: © 2025

PY - 2025/8

Y1 - 2025/8

N2 - Eutectic Nb-18.7Si alloys with different ceramic nanoparticle addition (Al2O3, TiC, SiC, 5 mol.-%), prepared by arc-melting, were heat-treated for 24 h at 1500 °C. Phase composition, microstructure transition and mechanical properties were investigated. The results show that the γ-Nb5Si3 and small Nb3Si phases from the as-cast alloy decomposed into α-Nb5Si3 and Nbss/α-Nb5Si3-eutectoids. Larger Nb3Si phases still existed after heat treatment. Additionally, after heat treatment the Nbss phases were interconnected to a continuous matrix, while silicides appeared coarsened and spherical while being uniformly distributed in the Nbss phase. This effect was most pronounced in the alloy with addition of Al2O3 nanoparticles, due to the ultrafine nano-scale lamellar structures of Nbss + α-Nb5Si3 in its as-cast condition. While the added nanoparticles had a strong effect on the initial microstructure of the as-cast state, they showed no noticeable effects like pinning of grain boundaries during heat treatment. A decrease in hardness was observed due to the coarsening of the microstructure and the reduced area fraction of silicide phases. However, the transformation to the coarser microstructure with a continuous Nbss matrix and spherical silicide phases seems to be effective in inhibiting crack propagation by promoting crack deflection and bridging over the Nbss phase.

AB - Eutectic Nb-18.7Si alloys with different ceramic nanoparticle addition (Al2O3, TiC, SiC, 5 mol.-%), prepared by arc-melting, were heat-treated for 24 h at 1500 °C. Phase composition, microstructure transition and mechanical properties were investigated. The results show that the γ-Nb5Si3 and small Nb3Si phases from the as-cast alloy decomposed into α-Nb5Si3 and Nbss/α-Nb5Si3-eutectoids. Larger Nb3Si phases still existed after heat treatment. Additionally, after heat treatment the Nbss phases were interconnected to a continuous matrix, while silicides appeared coarsened and spherical while being uniformly distributed in the Nbss phase. This effect was most pronounced in the alloy with addition of Al2O3 nanoparticles, due to the ultrafine nano-scale lamellar structures of Nbss + α-Nb5Si3 in its as-cast condition. While the added nanoparticles had a strong effect on the initial microstructure of the as-cast state, they showed no noticeable effects like pinning of grain boundaries during heat treatment. A decrease in hardness was observed due to the coarsening of the microstructure and the reduced area fraction of silicide phases. However, the transformation to the coarser microstructure with a continuous Nbss matrix and spherical silicide phases seems to be effective in inhibiting crack propagation by promoting crack deflection and bridging over the Nbss phase.

KW - AlO

KW - Heat treatment

KW - Microstructure

KW - Nanoparticle

KW - Nb-Si based alloy

KW - SiC

KW - TiC

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U2 - 10.1016/j.ijrmhm.2025.107170

DO - 10.1016/j.ijrmhm.2025.107170

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AN - SCOPUS:105001541382

VL - 130

JO - International Journal of Refractory Metals and Hard Materials

JF - International Journal of Refractory Metals and Hard Materials

SN - 0263-4368

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ER -

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